Optical and spin coherence of Er spin qubits in epitaxial cerium dioxide on silicon

Crystal field split energy levels of the 4I15/2 and 4I13/2 multiplets of Er3+ ions in CeO2.
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npj Quantum Information, Published online: 20 November 2024; doi:10.1038/s41534-024-00903-z

Robust spin-photon interfaces with optical transitions in the telecommunication band are essential for quantum networking technologies. Erbium (Er) ions are the ideal candidate with environmentally protected transitions in telecom-C band.

Finding the right technologically compatible host material to enable long-lived spins remains a major hurdle.

A team of researchers has introduced a new platform based on Er ions in cerium dioxide (CeO2) as a nearly-zero nuclear spin environment (0.04%) epitaxially grown on silicon, offering silicon compatibility for opto-electrical devices.

Their studies focused on Er3+ ions and showed a narrow homogeneous linewidth of 440 kHz with an optical coherence time of 0.72 μs at 3.6 K. The reduced nuclear spin noise enables a slow spin-lattice relaxation with a spin relaxation time up to 2.5 ms and an electron spin coherence time of 0.66 μs (in the isolated ion limit) at 3.6 K.

These findings highlight the potential of Er3+:CeO2 platform for quantum networks applications.

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